arXiv:2410.06422cs.LGcond-mat.mtrl-sci2024-10被引 2

用概率模型预测电池衰减,还能给出可信度评估。

Predicting Battery Capacity Fade Using Probabilistic Machine Learning Models With and Without Pre-Trained Priors

  • 采用贝叶斯方法构建三种概率模型,量化预测不确定性
  • 预训练的结构化高斯过程比神经网络更准且不确定性更优
  • 适合需可靠决策的电池健康监测场景

锂离子电池是推动移动电子、电动汽车和可再生能源存储革命的关键储能技术。容量保持率是评估电池是否接近寿命终点的重要性能指标。机器学习(ML)能基于历史数据预测容量退化,但其预测可信度在关乎重大决策时至关重要。本研究探索了全贝叶斯机器学习在电池健康预测中的有效性,重点量化预测不确定性。具体实施了三种概率性机器学习方法:标准高斯过程(GP)、结构化高斯过程(sGP)和全贝叶斯神经网络(BNN)。传统上,GP和sGP的超参数仅从单个样本中学习,而BNN通常在现有数据集上预训练以学习权重分布。这种差异使BNN在有充足训练数据时更具优势。然而,我们发现可将预训练用于GP和sGP,以学习超参数先验分布;其中,预训练的sGP在预测精度上与BNN相当,并实现了更好的不确定性估计。该方法为可利用历史数据学习概率模型先验的广泛场景提供了框架。

原文摘要 · Abstract (English)

Lithium-ion batteries are a key energy storage technology driving revolutions in mobile electronics, electric vehicles and renewable energy storage. Capacity retention is a vital performance measure that is frequently utilized to assess whether these batteries have approached their end-of-life. Machine learning (ML) offers a powerful tool for predicting capacity degradation based on past data, and, potentially, prior physical knowledge, but the degree to which an ML prediction can be trusted is of significant practical importance in situations where consequential decisions must be made based on battery state of health. This study explores the efficacy of fully Bayesian machine learning in forecasting battery health with the quantification of uncertainty in its predictions. Specifically, we implemented three probabilistic ML approaches and evaluated the accuracy of their predictions and uncertainty estimates: a standard Gaussian process (GP), a structured Gaussian process (sGP), and a fully Bayesian neural network (BNN). In typical applications of GP and sGP, their hyperparameters are learned from a single sample while, in contrast, BNNs are typically pre-trained on an existing dataset to learn the weight distributions before being used for inference. This difference in methodology gives the BNN an advantage in learning global trends in a dataset and makes BNNs a good choice when training data is available. However, we show that pre-training can also be leveraged for GP and sGP approaches to learn the prior distributions of the hyperparameters and that in the case of the pre-trained sGP, similar accuracy and improved uncertainty estimation compared to the BNN can be achieved. This approach offers a framework for a broad range of probabilistic machine learning scenarios where past data is available and can be used to learn priors for (hyper)parameters of probabilistic ML models.

电池预测概率建模不确定性估计

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