用AI模型快速解析高应变率下软材料的力学特性
Transformer-Based Inverse Microrheology for Experimental Mechanics at Ultra-High Strain Rates
- 用Transformer网络直接从气泡动态数据推断材料参数
- 比传统方法快数十倍,误差小于5%且无需迭代优化
- 适合研究高速变形下的水凝胶、聚合物等软材料
传统流变工具在超高速加载条件(>1000 s⁻¹)下受限于时空分辨率、加载速率和侵入性。最近发展的惯性微气泡流变法(IMR)利用激光诱导惯性空化(LIC)动态扰动周围材料,可探测极端条件下的非线性粘弹性。但传统IMR依赖计算成本高的迭代反演,限制了其扩展性和实时应用。本文提出基于Transformer的气泡动力学框架(BDT),融合物理驱动的空化模拟与神经网络,直接从时间分辨的气泡半径演化曲线预测粘弹性参数,无需迭代优化。该模型使用基于Keller-Miksis方程的合成数据训练,并通过水凝胶和黏性聚合物溶液的实验激光空化数据验证。结果表明,该AI框架与先前IMR方法高度一致,同时显著加速本构参数推断。实验进一步展示其在从黏性液体到多种粘弹性水凝胶的宽范围软材料中,表征高应变率下的速率依赖行为的能力。
原文摘要 · Abstract (English)
Traditional rheological tools are often limited in characterizing soft materials under ultra-high strain-rate loading conditions (> 1000 s^-1) due to constraints in spatiotemporal resolution, loading rate, and invasiveness. Recently, inertial microcavitation rheometry (IMR), which utilizes laser-induced inertial cavitation (LIC) to dynamically deform surrounding materials, has emerged as a powerful experimental mechanics technique for probing nonlinear viscoelastic properties under extreme loading conditions. However, conventional IMR relies on computationally expensive iterative inverse fitting procedures, limiting its scalability and real-time applicability. Here, we introduce a new AI-enhanced experimental mechanics framework, called Bubble Dynamics Transformer (BDT), that integrates physics-based cavitation simulations with Transformer neural network architectures to achieve rapid inverse characterization of soft material viscoelasticity from experimentally measured bubble dynamics. The proposed framework directly predicts viscoelastic material parameters from time-resolved bubble radius evolution curves without iterative optimization. The BDT is trained using synthetic datasets generated from physics-based Keller--Miksis cavitation simulations and validated using experimental laser-induced cavitation data obtained from hydrogels and viscous polymer solutions. The proposed AI-driven framework demonstrates excellent agreement with our previous IMR while substantially accelerating constitutive parameter inference. Experimental demonstrations further reveal the capability of the framework to characterize rate-dependent material behavior across a wide range of soft materials, from viscous liquids to various viscoelastic hydrogels, at ultra-high strain rates.
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