用概率模型预测锂电池长期衰减,还能给出不确定度估计。
BattVAE-GP: Generative Modeling of Long-Horizon Battery Degradation with Uncertainty Quantification

- 先用变分自编码器提取衰减特征,再用高斯过程建模潜空间动态。
- 在未见充电速率下仍能准确预测电压-容量演化轨迹。
- 适合需要可靠预测与不确定性分析的电池健康评估场景。
长期基于物理的锂电池衰减模拟虽具机制洞察力,但计算成本高,难以密集探索长期循环下的工况。本文提出混合物理-概率学习框架BattVAE-GP,用于对未知充电速率下的锂离子电池衰减轨迹进行代理建模。首先利用PyBaMM中的DFN/P2D电化学模型生成周期解析的衰减数据,并将其转化为容量对齐的电压与导数特征,经变分自编码器(VAE)编码至二维潜空间;该潜空间按循环进程与充电制度组织衰减轨迹。随后在潜空间中训练稀疏多任务高斯过程(GP),以循环数和C-rate为输入,实现潜动态的连续插值并提供后验不确定度估计。在协议级留出评估中,潜空间GP能准确恢复未见C-rate的轨迹,且不确定度行为与训练数据支持范围一致;当查询未见内部C-rate时,模型生成的潜轨迹仍保持在邻近仿真协议之间的一致位置。通过冻结的VAE解码器将GP预测的潜状态解码,得到平滑的电压-容量演化;同时通过辅助潜空间到健康状态(SOH)预测器进行蒙特卡洛传播,获得带不确定性的SOH估计。该框架计算高效且具备不确定性感知能力,为拓展电池健康预测至更丰富工况及未来仿真-实验融合提供结构化基础。
原文摘要 · Abstract (English)
Long-horizon physics-based simulations of battery degradation provide mechanistic insight but remain computationally expensive, limiting their use for dense exploration of operating conditions over extended cycle life. Here, we propose a hybrid physics-probabilistic learning framework for surrogate modeling of lithium-ion battery degradation trajectories at unseen charging rates. Cycle-resolved degradation data generated with a DFN/P2D electrochemical model in PyBaMM are first transformed into capacity-aligned voltage and derivative features and encoded using a Variational Autoencoder (VAE). The resulting two-dimensional latent space organizes degradation trajectories according to both cycle progression and charging protocol. A sparse multitask Gaussian process (GP) is then trained in this latent space using cycle number and C-rate as input variables, providing continuous interpolation of latent degradation dynamics together with posterior uncertainty estimates. Under protocol-level holdout evaluation, the latent-space GP accurately recovers unseen C-rate trajectories and exhibits uncertainty behavior consistent with the support of the training data. When queried at unseen interior C-rates, the model generates latent trajectories that remain coherently positioned between neighboring simulated protocols. Decoding the GP-predicted latent states through the frozen VAE decoder yields smooth voltage-capacity evolution, while Monte Carlo propagation of the GP latent posterior through an auxiliary latent to State of Health (SOH) predictor provides uncertainty-aware SOH estimates. The proposed BattVAE-GP framework therefore offers a computationally efficient and uncertainty-aware surrogate for long-horizon degradation modeling, providing a structured basis for extending battery health prediction toward richer operating conditions and future simulation-experiment fusion.
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